Magnetic excitations probed by inelastic scanning tunneling spectroscopy, from thin films to single atoms

W. Wulfhekel

Physikalisches Institut, Universität Karlsruhe, Wolfgang-Gaede-Str. 1, 76131Karlsruhe, Germany

 

When passing an electric current through a magnetic material, magnetic excitations can be created.  In these inelastic scattering events, the electron spin of the current is flipped and angular momentum is transferred to the magnetic system in form of a magnon.  Energy is required for such excitations, making inelastic scanning tunneling spectroscopy (ISTS) the method of choice to study these excitations in nanoscale systems. We have successfully applied ISTS to investigate the nature of the inelastic spin-torque effect, to obtain magnon dispersions in thin films with precision similar to neutron scattering and to measure the magnetic anisotropy of single magnetic atoms and clusters.

The results on magnetic excitations in bulk Fe and thin films of Co on Cu(100) and Cu(111) will be presented and discussed. They show that the probability of current-assisted magnon creation is proportional to the spin polarization of the local density of states of the sample. They also indicate that magnon excitation in magnetic tunnel junctions should not be neglected, as most minority electrons scatter inelastically leading to magnon creation. The experiments further identify the interaction responsible for the spin scattering to be the RKKY interaction.

A thickness-dependent study of inelastic tunneling spectra of thin films of Co on Cu(100) allowed experimental determination of the magnon dispersion in fcc Co with high resolution. The results show no deviation from bulk behavior down to the film thickness of 8 monolayers. The determined magnon stiffness is 667±3 eV·Å2.

The high lateral resolution of the ISTS enables addressing single atoms on surfaces. Further, atoms may be laterally manipulated with the STM tip to form well-defined atomic clusters of magnetic material. Using both techniques combined, the magnetic anisotropies of single atoms, dimers and trimers of Fe and Co on Pt(111) were determined. The results are compared to XMCD data and theoretical calculations.